Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture? Academic Article uri icon

Overview

abstract

  • Fano resonances and Rabi splittings are routinely reported in the scientific literature. Asymmetric resonance lineshapes are usually associated with Fano resonances, and two split peaks in the spectrum are often attributed to a Rabi splitting. True Fano resonances and Rabi splittings are unequivocal signatures of coherent coupling between subsystems. However, can the same spectral lineshapes characterizing Fano resonances and Rabi splittings arise from a purely incoherent sum of intensities? Here we answer this question through experiments with a tunable Fabry-PĂ©rot cavity containing a CsPbBr3 perovskite crystal. By measuring the transmission and photoluminescence of this system using microscope objectives with different numerical aperture (NA), we find that even a modest NA = 0.4 can artificially generate Fano resonances and Rabi splittings. We furthermore show that this modest NA can obscure the anticrossing of a bona fide strongly coupled light-matter system. Through transfer matrix calculations we confirm that these spectral artifacts are due to the incoherent sum of transmitted intensities at different angles captured by the NA. Our results are relevant to the wide nanophotonics community, characterizing dispersive optical systems with high numerical aperture microscope objectives. We conclude with general guidelines to avoid pitfalls in the characterization of such optical systems.

publication date

  • May 4, 2021

Identity

PubMed Central ID

  • PMC8155561

Scopus Document Identifier

  • 85065094161

Digital Object Identifier (DOI)

  • 10.1021/acs.jpcc.9b01406

PubMed ID

  • 34056036

Additional Document Info

volume

  • 8

issue

  • 5